Consistency between ARPES and STM measurements on SmB6

Publication information:

Matt, C., Pirie, H., Soumyanarayanan, A., He, Y., Yee, M., Chen, P., Liu, Y., Larson, D., Paz, W., Palacios, J., & others. (2020). Consistency between ARPES and STM measurements on SmB6. Physical Review B, 101(8), 085142. https://doi.org/10.1103/PhysRevB.101.085142

Abstract

The Kondo insulator SmB6 has emerged as a primary candidate for exotic quantum phases, due to the predicted formation of strongly correlated, low-velocity topological surface states and corresponding high Fermi-level density of states. However, measurements of the surface-state velocity in SmB6 differ by orders of magnitude, depending on the experimental technique used. Here we reconcile two techniques, scanning tunneling microscopy (STM) and angle-resolved photoemission spectroscopy (ARPES), by accounting for surface band bending on polar terminations. Using spatially resolved scanning tunneling spectroscopy, we measure a band shift of ∼20 meV between full-Sm and half-Sm terminations, in qualitative agreement with our density-functional theory calculations of the surface charge density. Furthermore, we reproduce the apparent high-velocity surface states reported by ARPES by simulating their observed spectral function as an equal-weight average over the two band-shifted domains that we image by STM. Our results highlight the necessity of local measurements to address inhomogeneously terminated surfaces or fabrication techniques to achieve uniform termination for meaningful large-area surface measurements of polar crystals such as SmB6.